期刊
TETRAHEDRON LETTERS
卷 49, 期 47, 页码 6650-6654出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.tetlet.2008.09.026
关键词
Three-component coupling reactions; Aldehyde-alkyne-amine; Propargylamines; PS-supported NHC-Ag(I); Solvent-free
资金
- National Natural Science Foundation of China [20572031, 20772043]
The development of a highly efficient, polystyrene-supported NHC-Ag(I) catalyst for the three-component coupling reactions of aldehydes, alkynes, and amines (A(3)-coupling) was described. In the presence of PS-NHC-Ag(I) (2 mol %). the A(3)-reactions were carried out at room temperature under solvent-free reaction conditions and the corresponding propargylamines were generated in good to excellent yields. Furthermore, the catalyst could be reused at least 12 times without a significant loss of its catalytic activity. (C) 2008 Published by Elsevier Ltd.
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