期刊
TETRAHEDRON LETTERS
卷 49, 期 27, 页码 4209-4212出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.tetlet.2008.04.162
关键词
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A novel organocatalytic highly enantioselective nitrocyclopropanation reaction of alpha,beta-unsaturated aldehydes is presented. The 1-nitro-2-formylcyclopropane derivatives synthesized from this catalytic transformation were converted to the corresponding beta-nitromethyl-acid esters, which are excellent precursors of GABA analogues such as Baclofen, by subsequent organocatalytic chemoselective ring-opening. (C) 2008 Elsevier Ltd. All rights reserved.
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