期刊
TETRAHEDRON
卷 65, 期 52, 页码 10882-10892出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.tet.2009.09.112
关键词
-
资金
- EPSRC
The regioselective synthesis of alkenylcyclanones by the oxidative radical cyclisation of malonyl radicals onto both allenes and an allylsilane is reported, along with the diastereoselective formation of [3.3.0]-bicyclic gamma-lactones from two of these alkenylcyclanones. Furthermore, the cyclisation of 3-,4- and 5-allenyl malonates on exposure to manganese(III) acetate under both oxidative and reductive termination conditions is reported. (C) 2009 Elsevier Ltd. All rights reserved.
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