期刊
TETRAHEDRON
卷 65, 期 33, 页码 6712-6719出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.tet.2008.10.060
关键词
Natural product; Alkaloid; Heck reaction; Carbonylation; Amidines
A strategy for a total synthesis of the marine alkaloid perophoramidine has been investigated. Key steps which have been tested include a tandem intramolecular Heck/carbonylation reaction and a stereoselective allylation of a pentacyclic delta-lactam to produce the C-4/20 vicinal quaternary centers having the requisite relative configuration of the metabolite. (C) 2008 Published by Elsevier Ltd.
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