期刊
SYNTHETIC METALS
卷 162, 期 1-2, 页码 95-101出版社
ELSEVIER SCIENCE SA
DOI: 10.1016/j.synthmet.2011.11.017
关键词
Single wall carbon nanotube; Fullerene; C-60; P3HT:PCBM; Hybrid; Organic photovoltaics
资金
- US Department of Energy [DE-FG36-08GO88008]
- US Department of Defense [DD-N000141110069]
The use of carbon nanotube-fullerene hybrid additives to the standard P3HT:PCBM blend bulk-heterojunction organic photovoltaic device is presented. The effects of incorporating single-wall carbon nanotubes, functionalized with linked C-60 molecules by amination on device characteristics are detailed. The concentration of the carbon nanotube-fullerene hybrid in the active layer blend was varied to ascertain their cumulative impact on device performance in terms of open circuit voltage, short circuit current, fill factor and efficiency. We found that decreasing the length of the carbon nanotubes to similar to 60 nm through fluorination and subsequent thermal treatment was beneficial in terms of eliminating shorted devices allowing much improved diode formation. A trend of improving device performance as a function of concentration of the carbon nanotube-hybrids in a heterojunction of P3HT:PCBM was observed. (C) 2011 Elsevier B.V. All rights reserved.
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