期刊
ADVANCED ENERGY MATERIALS
卷 6, 期 1, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/aenm.201501659
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资金
- National Science Foundation (CAREER Award) [CBET-1254662, IIP-1431010]
- DuPont Young Professor Award
A new series of organic salts with selective near-infrared (NIR) harvesting to 950 nm is reported, and anion selection and blending is demonstrated to allow for fine tuning of the open-circuit voltage. Extending photoresponse deeper into the NIR is a significant challenge facing small molecule organic photovoltaics, and recent demonstrations have been limited by open-circuit voltages much lower than the theoretical and practical limits. This work presents molecular design strategies that enable facile tuning of energy level alignment and open-circuit voltages in organic salt-based photovoltaics. Anions are also shown to have a strong influence on exciton diffusion length. These insights provide a clear route toward achieving high efficiency transparent and panchromatic photovoltaics, and open up design opportunities to rapidly tailor molecules for new donor-acceptor systems.
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