期刊
ACS CATALYSIS
卷 5, 期 8, 页码 4643-4667出版社
AMER CHEMICAL SOC
DOI: 10.1021/acscatal.5b00524
关键词
oxygen reduction reaction; oxygen electrocatalysis; catalysts; mechanisms; reaction pathways; alkaline
资金
- Advanced Energy Storage Research Programme, Institute of Materials Research and Engineering (IMRE) of the Agency for Science, Technology and Research (A*STAR) [IMRE/12-2P0503, IMRE/12-2P0504]
The oxygen reduction reaction (ORR) is an important electrode reaction for energy storage and conversion devices based on oxygen electrocatalysis. This paper introduces the thermodynamics, reaction kinetics, reaction mechanisms, and reaction pathways of ORR in aqueous alkaline media. Recent advances of the catalysts for ORR were extensively reviewed, including precious metals, nonmetal-doped carbon, carbon-transition metal hybrids, transition metal oxides with spinel and perovskite structures, and so forth. The applications of those ORR catalysts to zinc-air batteries and alkaline fuel cells were briefly introduced. A concluding remark summarizes the current status of the reaction pathways, advanced catalysts, and the future challenges of the research and development of ORR
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