期刊
ACS CATALYSIS
卷 5, 期 12, 页码 7194-7198出版社
AMER CHEMICAL SOC
DOI: 10.1021/acscatal.5b02411
关键词
copper catalysis; C-N bond formation; quinolines; azoles; C2 functionalization
资金
- National Nature Science Foundation of China [U1504210, 21172056, 21372065]
- Program for Changjiang Scholars and Innovative Research Team in University [IRT1061]
- China Postdoctoral Science Foundation [2015M572110]
- Science and Technology Plan Projects of Henan Province [15A150030]
Here, we report the copper-catalyzed C2 selective cross-dehydrogenative C-N bond formation of azines with azoles. This straightforward method enables us to address the key limitation of prior N-O activation strategy in C2 amination of azines. The wide substrate scope, high functional group tolerance, and ease of operation of the present method are expected to promote its potential application in synthetic chemistry.
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