4.8 Article

Accessing the transport properties of graphene and its multilayers at high carrier density

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NATL ACAD SCIENCES
DOI: 10.1073/pnas.1018388108

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  1. MEXT (Ministry of Education, Culture, Sports, Science, Technology)
  2. JST (Japan Science and Technology Agency)
  3. MaNEP (Materials with Novel Electronic Properties)
  4. Swiss National Science Foundation [200021_121569]
  5. Swiss National Science Foundation (SNF) [200021_121569] Funding Source: Swiss National Science Foundation (SNF)
  6. Grants-in-Aid for Scientific Research [23656011, 21224009] Funding Source: KAKEN

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We present a comparative study of high carrier density transport in mono-, bi-, and trilayer graphene using electric double-layer transistors to continuously tune the carrier density up to values exceeding 10(14) cm(-2). Whereas in monolayer the conductivity saturates, in bi- and trilayer filling of the higher-energy bands is observed to cause a nonmonotonic behavior of the conductivity and a large increase in the quantum capacitance. These systematic trends not only show how the intrinsic high-density transport properties of graphene can be accessed by field effect, but also demonstrate the robustness of ion-gated graphene, which is crucial for possible future applications.

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