期刊
POLYMER CHEMISTRY
卷 5, 期 11, 页码 3617-3623出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4py00073k
关键词
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资金
- NSF [CHE-1305773]
- National Research Foundation of Korea (NRF) - Korea Ministry of Science, ICT & Future Planning (MSIP) [2010-0018290]
- BK21 Plus Program in SNU Chemical Engineering
- WCU Program of Chemical Convergence for Energy and Environment [R31-10013]
A novel synthetic and processing strategy for converting elemental sulfur into polymeric and nanocomposite materials is reported. We describe a facile one-pot reaction using elemental sulfur and oleylamine as comonomers to prepare high sulfur content copolymers and lead sulfide nanoparticle (PbS NP) nanocomposites. This process enables the preparation of solution processable copolymers and nanocomposites, where the loading and dispersion of PbS NP inclusions could be precisely controlled. We demonstrate the dual roles of oleylamine with sulfur for both the copolymerization of sulfur copolymers as well as the in situ synthesis of PbS NPs in a one-pot fashion.
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