期刊
CHEMICAL SCIENCE
卷 6, 期 4, 页码 2158-2165出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4sc01945h
关键词
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资金
- National Science Foundation Graduate Research Fellowship Program [DGE 1106401]
- NSF Triangle MRSEC [DMR-1121107]
- Duke University
Force reactive functional groups, or mechanophores, have emerged as the basis of a potential strategy for sensing and countering stress-induced material failure. The general utility of this strategy is limited, however, because the levels of mechanophore activation in the bulk are typically low and observed only under large, typically irreversible strains. Strategies that enhance activation are therefore quite useful. Molecular-level design principles by which to engineer enhanced mechanophore activity are reviewed, with an emphasis on quantitative structure-activity studies determined for a family of gem-dihalocyclopropane mechanophores.
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