4.8 Article

Imaging Ultrafast Demagnetization Dynamics after a Spatially Localized Optical Excitation

期刊

PHYSICAL REVIEW LETTERS
卷 112, 期 21, 页码 -

出版社

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.112.217203

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资金

  1. German Bundesministerium fur Bildung und Forschung [05K10KTB/FSP-301]
  2. FERMI project of Elettra-Sincrotrone Trieste
  3. Ministry of University and Research [FIRB-RBAP045JF2, FIRB-RBAP06AWK3]
  4. DFG [SFB 925]
  5. CNRS through the PEPS SASELEX
  6. French ANR via the FEMTO-X-MAG project
  7. LabEx PALM through the RAMSES project

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Ultrashort, coherent x-ray pulses of a free-electron laser are used to holographically image the magnetization dynamics within a magnetic domain pattern after creation of a localized excitation via an optical standing wave. We observe a spatially confined reduction of the magnetization within a couple of hundred femtoseconds followed by its slower recovery. Additionally, the experimental results show evidence of a spatial evolution of magnetization, which we attribute to ultrafast transport of nonequilibrium spin-polarized electrons for early times and to a fluence-dependent remagnetization rate for later times.

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