期刊
PHYSICAL REVIEW LETTERS
卷 112, 期 15, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.112.155504
关键词
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资金
- Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]
- Center for Nanoscale Control of Geologic CO2, a U.S. DOE Energy Frontier Research Center [DE-AC02-05CH11231]
- KSU startup funds
- Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]
We use analytic theory and computer simulation to study patterns formed during the growth of two-component assemblies in two and three dimensions. We show that these patterns undergo a nonequilibrium phase transition, at a particular growth rate, between mixed and demixed arrangements of component types. This finding suggests that principles of nonequilibrium statistical mechanics can be used to predict the outcome of multicomponent self-assembly, and suggests an experimental route to the self-assembly of multicomponent structures of a qualitatively defined nature.
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