4.8 Article

48Ca+249Bk Fusion Reaction Leading to Element Z=117: Long-Lived α-Decaying 270Db and Discovery of 266Lr

期刊

PHYSICAL REVIEW LETTERS
卷 112, 期 17, 页码 -

出版社

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.112.172501

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资金

  1. German BMBF [05P12UMFNE]
  2. Helmholtz association [VH-NG-723]
  3. Australian Research Council
  4. Swedish Research Council
  5. U.S. Department of Energy by LLNL [DE-AC52-07NA27344]
  6. Laboratory Directed Research and Development Program at LLNL [11-ERD-011]
  7. Helmholtz Institute Mainz
  8. Office of Science, U.S. Department of Energy
  9. U.S. DOE [DE-AC05-00OR22725]
  10. Vanderbilt DOE [DE-FG05-88ER40407]
  11. UK Science and Technology Funding Council (STFC)
  12. U.S. Department of Energy, Office of Science, Nuclear Physics, Low Energy Physics Program, through the Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]
  13. STFC [ST/F012039/1, ST/J000094/1] Funding Source: UKRI
  14. Science and Technology Facilities Council [ST/F012039/1, ST/J000094/1] Funding Source: researchfish

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The superheavy element with atomic number Z = 117 was produced as an evaporation residue in the Ca-48 + Bk-249 fusion reaction at the gas-filled recoil separator TASCA at GSI Darmstadt, Germany. The radioactive decay of evaporation residues and their alpha-decay products was studied using a detection setup that allowed measuring decays of single atomic nuclei with half-lives between sub-mu s and a few days. Two decay chains comprising seven a decays and a spontaneous fission each were identified and are assigned to the isotope (294)117 and its decay products. A hitherto unknown alpha-decay branch in (270)Db (Z = 105) was observed, which populated the new isotope Lr-266 (Z = 103). The identification of the long-lived (T-1/2 = 1.0(-0.4)(+1.9) h) alpha-emitter (270)Db marks an important step towards the observation of even more long-lived nuclei of superheavy elements located on an island of stability.

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