期刊
PHYSICAL REVIEW LETTERS
卷 113, 期 4, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.113.043901
关键词
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资金
- Russian Foundation for Basic Research
- Welch Foundation [A-1801]
- Russian Science Foundation [14-12-00772]
- Russian Quantum Center fellowship
- Russian Science Foundation [14-12-00772] Funding Source: Russian Science Foundation
Ultrafast ionization dynamics within the field half cycle is shown to be the key physical factor that controls the properties of optical nonlinearity as a function of the carrier wavelength and intensity of a driving laser field. The Schrodinger-equation analysis of a generic hydrogen quantum system reveals universal tendencies in the wavelength dependence of optical nonlinearity, shedding light on unusual properties of optical nonlinearities in the midinfrared. For high-intensity low-frequency fields, free-state electrons are shown to dominate over bound electrons in the overall nonlinear response of a quantum system. In this regime, semiclassical models are shown to offer useful insights into the physics behind optical nonlinearity.
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