期刊
PHYSICAL REVIEW LETTERS
卷 110, 期 1, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.110.018304
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资金
- Institut Universitaire de France
- European Research Council under the European Union's Seventh Framework Programme (FP7)
- ERC [258803]
- European Research Council (ERC) [258803] Funding Source: European Research Council (ERC)
The nonlinear rheology of a soft glassy material is captured by its constitutive relation, shear stress versus shear rate, which is most generally obtained by sweeping up or down the shear rate over a finite temporal window. For a huge amount of complex fluids, the up and down sweeps do not superimpose and define a rheological hysteresis loop. By means of extensive rheometry coupled to time-resolved velocimetry, we unravel the local scenario involved in rheological hysteresis for various types of well-studied soft materials. We introduce two observables that quantify the hysteresis in macroscopic rheology and local velocimetry, respectively, as a function of the sweep rate delta t(-1). Strikingly, both observables present a robust maximum with delta t, which defines a single material-dependent time scale that grows continuously from vanishingly small values in simple yield stress fluids to large values for strongly time-dependent materials. In line with recent theoretical arguments, these experimental results hint at a universal time scale-based framework for soft glassy materials, where inhomogeneous flows characterized by shear bands and/or pluglike flow play a central role. DOI: 10.1103/PhysRevLett.110.018304
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