期刊
PHYSICAL REVIEW LETTERS
卷 110, 期 24, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.110.247401
关键词
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资金
- Funding Program for World-Leading Innovative R&D on Science and Technology (FIRST)
- International Institute for Carbon Neutral Energy Research (WPI-I2CNER)
- Ministry of Education, Culture, Sports, Science and Technology
We demonstrate an organic molecule with an energy gap between its singlet and triplet excited states of almost zero (Delta E-ST similar to 0 eV). Such separation was realized through proper combination of an electron-donating indolocarbazole group and a diphenyltriazine electron-accepting moiety. Calculated and measured Delta E-ST were 0.003 and 0.02 eV, respectively. A total photoluminescence efficiency of 59% +/- 2% with 45% +/- 2% from a delayed component and 14% +/- 2% from a prompt component was obtained for a doped film. Organic light emitting diodes containing this molecule as an emitting dopant exhibited an unexpectedly high external electroluminescence efficiency of eta(EQE) = 14% +/- 1%.
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