期刊
PHYSICAL REVIEW LETTERS
卷 108, 期 22, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.108.225506
关键词
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资金
- NSF [OCI-0753335, OCI-0821678, OCI-1053575, OCI-1007115, DGE-07-07425, CHE-0910943, CHE-0719089]
- DOE
- NIH [S10-RR029030-01]
- Office of Advanced Cyberinfrastructure (OAC)
- Direct For Computer & Info Scie & Enginr [1007115, 1148443] Funding Source: National Science Foundation
- Office of Advanced Cyberinfrastructure (OAC)
- Direct For Computer & Info Scie & Enginr [0753335] Funding Source: National Science Foundation
It has been demonstrated recently that supercooled liquids sharing simple structural features (e. g. pair distribution functions) may exhibit strikingly distinct dynamical behavior. Here we show that a more subtle structural feature correlates with relaxation times in three simulated systems that have nearly identical radial distribution functions but starkly different dynamical behavior. In particular, for the first time we determine the thermodynamic point-to-set length scale in several canonical model systems and demonstrate the quantitative connection between this length scale and the growth of relaxation times. Our results provide clues necessary for distinguishing competing theories of the glass transition.
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