4.8 Article

Spectral Properties of Correlated Materials: Local Vertex and Nonlocal Two-Particle Correlations from Combined GW and Dynamical Mean Field Theory

期刊

PHYSICAL REVIEW LETTERS
卷 109, 期 22, 页码 -

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AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.109.226401

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资金

  1. French ANR under project SURMOTT
  2. GENCI/IDRIS Orsay [1393]
  3. DFG [FOR 1346]
  4. Swiss National Science Foundation [PP0022-118866]
  5. Swiss National Science Foundation (SNF) [PP0022_118866] Funding Source: Swiss National Science Foundation (SNF)

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We present a fully self-consistent combined GW and dynamical mean field (DMFT) study of the extended two-dimensional Hubbard model. The inclusion of the local dynamical vertex stemming from the DMFT self-energy and polarization is shown to cure the known problems of self-consistent GW. We calculate momentum-resolved spectral functions, two-particle polarizations, and electron-loss spectra, as well as the effective dynamical interaction induced by nonlocal screening. The momentum-dependence introduced by GW into the extended DMFT description leads to a narrowing of the quasiparticle width and more pronounced Hubbard bands in the metallic regime as one approaches the charge-ordering transition. It further affects the shape of collective modes, giving rise to dispersive plasmon-like long-wavelength and stripe modes.

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