期刊
PHYSICAL REVIEW LETTERS
卷 108, 期 15, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.108.153003
关键词
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资金
- DOE, Office of Science, Basic Energy Science, Chemical, Geosciences, and Biological Divisions
- MEXT
- JST
- JSPS, Japan
- MIUR Italy [FIRB-RBAP045JF2, FIRB-RBAP06AWK3]
- Swedish Research Council (VR)
- Grants-in-Aid for Scientific Research [23550017] Funding Source: KAKEN
We have performed x-ray two-photon photoelectron spectroscopy using the Linac Coherent Light Source x-ray free-electron laser in order to study double core-hole (DCH) states of CO2, N2O, and N-2. The experiment verifies the theory behind the chemical sensitivity of two-site DCH states by comparing a set of small molecules with respect to the energy shift of the two-site DCH state and by extracting the relevant parameters from this shift.
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