期刊
PHYSICAL REVIEW LETTERS
卷 108, 期 6, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.108.063009
关键词
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资金
- MICINN [FIS2010-15127, ACI2008-0777, CSD 2007-00010]
- ERA [PIM2010EEC-00751]
- European grant MC-ITN CORINF
- European grant MC-RG ATTOTREND
- European COST Action [CM0702]
- European Research Council XCHEM [290853]
- European Research Council (ERC) [290853] Funding Source: European Research Council (ERC)
We investigate the use of UV-pump-UV-probe schemes to trace the evolution of nuclear wave packets in excited molecular states by analyzing the asymmetry of the electron angular distributions resulting from dissociative ionization. The asymmetry results from the coherent superposition of gerade and ungerade states of the remaining molecular ion in the region where the nuclear wave packet launched by the pump pulse in the neutral molecule is located. Hence, the variation of this asymmetry with the time delay between the pump and the probe pulses parallels that of the moving wave packet and, consequently, can be used to clock its field-free evolution. The performance of this method is illustrated for the H-2 molecule.
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