4.8 Article

Multiphoton Above Threshold Effects in Strong-Field Fragmentation

期刊

PHYSICAL REVIEW LETTERS
卷 109, 期 16, 页码 -

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AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.109.163003

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  1. Danish Research Council [10-085430]
  2. ERC-StG [277767-TDMET]
  3. Chemical Sciences, Geosciences, and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy
  4. Kansas State University

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We present a study of multiphoton dissociative ionization from molecules. By solving the time-dependent Schrodinger equation for H-2(+) and projecting the solution onto double continuum scattering states, we observe the correlated electron-nuclear ionization dynamics in detail. We show-for the first time-how multiphoton structure prevails as long as one accounts for the energies of all the fragments. Our current work provides a new avenue to analyze strong-field fragmentation that leads to a deeper understanding of the correlated molecular dynamics.

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