期刊
PHYSICAL REVIEW LETTERS
卷 107, 期 25, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.107.257402
关键词
-
资金
- European Commission [MRTN-CT-2006-035859]
- Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences
We present evidence for the generation of free carriers in aggregated single-wall carbon nanotubes by photoexcitation in the energetic range of the pi ->pi* transition associated with the M saddle point of the graphene lattice. The underlying broad absorption culminating at 4.3 eV can be fit well with a Fano line shape that describes strong coupling of a saddle-point exciton to an underlying free electron-hole pair continuum. Moreover, it is demonstrated that transitions in this energetic region autoionize into the continuum by detecting features unique to the presence of free charges in the transient transmission spectra of the continuum-embedded second sub-band exciton, S(2).
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