期刊
PHYSICAL REVIEW LETTERS
卷 106, 期 15, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.106.153004
关键词
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资金
- Swedish Research Council (VR)
- Carl Tryggers Stiftelse (CTS)
Resonant inelastic soft x-ray scattering (RIXS) spectra excited at the 1 sigma(g) -> 3 sigma(u) resonance in gas-phase O-2 show excitations due to the nuclear degrees of freedom with up to 35 well-resolved discrete vibronic states and a continuum due to the kinetic energy distribution of the separated atoms. The RIXS profile demonstrates spatial quantum beats caused by two interfering wave packets with different momenta as the atoms separate. Thomson scattering strongly affects both the spectral profile and the scattering anisotropy.
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