4.8 Article

Brownian Fluctuations and Heating of an Optically Aligned Gold Nanorod

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PHYSICAL REVIEW LETTERS
卷 107, 期 3, 页码 -

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AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.107.037401

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  1. Foundation for Fundamental Research on Matter (FOM)
  2. Dutch Organization for Scientific Research (NWO)
  3. ERC

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We present the first quantitative measurements of the torque exerted on a single gold nanorod in a polarized three-dimensional optical trap. We determined the torque both by observing the time-averaged orientation distribution and by measuring the dynamics of the rotational Brownian fluctuations. The measurements are in good agreement with calculations, where the temperature profile around the hot nanorod gives rise to a reduced, effective viscosity. The maximum torque on a 60 nm x 25 nm nanorod was 100 pN . nm, large enough to address single-molecule processes in soft and biological matter.

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