期刊
PHYSICAL REVIEW LETTERS
卷 107, 期 16, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.107.166102
关键词
-
资金
- Deutsche Forschungsgemeinschaft via Nanosystems Initiative Munich
- [GE2214/1]
The framework for deriving tensorial interfacial dielectric profiles from bound charge distributions is established and applied to molecular dynamics simulations of water at hydrophobic and hydrophilic surfaces. In conjunction with a modified Poisson-Boltzmann equation, the trend of experimental double-layer capacitances is well reproduced. We show that the apparent Stern layer can be understood in terms of the dielectric profile of pure water.
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