期刊
PHYSICAL REVIEW LETTERS
卷 106, 期 3, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.106.033402
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资金
- Deutsche Forschungsgemeinschaft
- Advanced Study Group of the Max-Planck-Society
- Fonds der chemischen Industrie
Electron-electron coincidence spectra of Ar-Kr clusters after photoionization have been measured. An electron with the kinetic energy range from 0 to approximately 1 eV is found in coincidence with the Ar 3s cluster photoelectron. The low kinetic energy electron can be attributed to an Ar + Kr+ + Kr+ final state which forms after electron transfer mediated decay. This autoionization mechanism results from a concerted transition involving three different atoms in a van der Waals cluster; it was predicted theoretically, but hitherto not observed.
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