4.8 Article

Attosecond Two-Photon Interferometry for Doubly Excited States of Helium

期刊

PHYSICAL REVIEW LETTERS
卷 107, 期 9, 页码 -

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AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.107.093005

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资金

  1. FWF-Austria [SFB016, P21141-N16]
  2. NSF
  3. NNSA of the U.S. DOE [DE-AC52-06NA25396]
  4. TACC [TG-PHY090031]

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We show that the correlation dynamics in coherently excited doubly excited resonances of helium can be followed in real time by two-photon interferometry. This approach promises to map the evolution of the two-electron wave packet onto experimentally easily accessible noncoincident single-electron spectra. We analyze the interferometric signal in terms of a semianalytical model which is validated by a numerical solution of the time-dependent two-electron Schrodinger equation in its full dimensionality.

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