4.8 Article

High Harmonic Spectroscopy of Multichannel Dynamics in Strong-Field Ionization

期刊

PHYSICAL REVIEW LETTERS
卷 104, 期 21, 页码 -

出版社

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.104.213601

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资金

  1. Leibniz SAW
  2. A. von Humboldt foundation
  3. ANR [ANR-08-JCJC-0029 HarMoDyn]
  4. EPSRC [EP/E036112/1] Funding Source: UKRI
  5. Engineering and Physical Sciences Research Council [EP/E036112/1] Funding Source: researchfish

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We perform high harmonic generation spectroscopy of aligned nitrogen molecules to characterize the attosecond dynamics of multielectron rearrangement during strong-field ionization. We use the spectrum and ellipticity of the harmonic light to reconstruct the relative phase between different ionization continua participating in the ionization, and thus determine the shape and location of the hole left in the molecule by strong-field ionization. Our interferometric technique uses transitions between the ionic states, induced by the laser field on the subcycle time scale.

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