期刊
PHYSICAL REVIEW LETTERS
卷 105, 期 23, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.105.233001
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资金
- Triangle de la Physique in France
- Swedish Research Council (VR)
- Carl Tryggers Stiftelse (CTS) foundation in Sweden
Dissociative nuclear motion in core-excited molecular states leads to a splitting of the fragment Auger lines: the Auger-Doppler effect. We present here for the first time experimental evidence for an Auger-Doppler effect following F1s -> a(1g)* inner-shell excitation by circularly polarized x rays in SF6. In spite of a uniform distribution of the dissociating S-F bonds near the polarization plane of the light, the intersection between the subpopulation of molecules selected by the core excitation with the cone of dissociation induces a strong anisotropy in the distribution of the S-F bonds that contributes to the scattering profile measured in the polarization plane.
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