期刊
PHYSICAL REVIEW LETTERS
卷 103, 期 8, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.103.087205
关键词
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资金
- NSF NIRT [ECS-0609469]
- Alexander von Humboldt Foundation
- Miller Institute
We have fabricated hybrid magnetic complexes from V atoms and tetracyanoethylene ligands via atomic manipulation with a cryogenic scanning tunneling microscope. Using tunneling spectroscopy we observe spin-polarized molecular orbitals as well as Kondo behavior. For complexes having two V atoms, the Kondo behavior can be quenched for different molecular arrangements, even as the spin-polarized orbitals remain unchanged. This is explained by variable spin-spin (i.e., V-V) ferromagnetic coupling through a single tetracyanoethylene (TCNE) molecule, as supported by density functional calculations.
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