期刊
PHYSICAL REVIEW LETTERS
卷 102, 期 4, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.102.043401
关键词
-
资金
- Deutsche Forschungsgemeinschaft
- Junta de Castilla y Leon
- Spanish MEC
- European Regional Development Fund [FIS2008-02490/FIS, GR120]
Caloric curves for sodium clusters with N=139 and 147 atoms show a fine structure near the solid-to-liquid transition. Neither of the two sizes exhibit surface melting. For N=139, diffusion of the surface vacancies is observed, which is not possible in the closed-shell N=147 cluster. A few kelvin above the peak in the heat capacity, N=139 is completely liquid. This is not the case for N=147. Here the inner 13 atoms remain nearly fixed up to several tens of kelvin above the melting temperature of the outer two layers. A simple physical reason is suggested for this unexpected behavior.
作者
我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。
推荐
暂无数据