4.8 Article

External magnetic field effects on a distorted kagome antiferromagnet

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PHYSICAL REVIEW LETTERS
卷 101, 期 10, 页码 -

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AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.101.107201

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资金

  1. U. S. DOE [DE-FG02-07ER45384]
  2. U. S. NSF [DMR-0454672]
  3. Japan Grant-in-Aid for Scientific Research [1905200]

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We report bulk magnetization, and elastic and inelastic neutron scattering measurements under an external magnetic field H on the weakly coupled distorted kagome system, Cu-2(OD)(3)Cl. Our results show that the ordered state below 6.7 K is a canted antiferromagnet and consists of large antiferromagnetic ac components and smaller ferromagnetic b components. By first-principles calculations and linear spin wave analysis, we present a simple spin Hamiltonian with nonuniform nearest neighbor exchange interactions resulting in a system of coupled spin trimers with a single-ion anisotropy that can qualitatively reproduce the spin dynamics of Cu-2(OD)(3)Cl.

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