4.8 Article

Order Parameter Description of Electrochemical-Hydrodynamic Interactions in Nanochannels

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PHYSICAL REVIEW LETTERS
卷 101, 期 18, 页码 -

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AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.101.184501

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A novel phase-field model is developed for the quantitative modeling of the complex electrochemical-hydrodynamic interactions in narrow fluidic confinements. Through an order parameter variation, this model captures the underlying excluded volume effects, solvation interactions, and preferential polarizabilities in a self-consistent fashion, without resorting to computationally prohibitive molecular dynamics simulations. Agreement with molecular dynamics predictions is found to be quantitative.

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