期刊
PHYSICAL REVIEW B
卷 89, 期 16, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.89.161406
关键词
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资金
- Deutsche Forschungsgemeinschaft [SFB 445]
- EU consortium REFreePerMag
- Office of Science, Office of Basic Energy Sciences of the US Department of Energy [DE-AC02-05CH11231]
The crystal structure of FePt nanoparticles of mean size of 6 nm produced by gas-phase condensation is characterized using a combination of high-resolution transmission electron microscopy (HRTEM) and high-angle annular dark field (HAADF) imaging in scanning transmission electron microscopy (STEM). These FePt nanoparticles are found to be chemically ordered, decahedral shaped, and Pt enriched at the surfaces. The experimentally determined crystallographic lattice constants and distribution of Fe and Pt atoms are compared with first-principles calculations of ordered decahedral FePt nanoparticles to confirm the discovery of a unique decahedral structure with Fe/Pt ordering and Pt surface segregation.
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