4.6 Article

Transient carrier dynamics in a Mott insulator with antiferromagnetic order

期刊

PHYSICAL REVIEW B
卷 89, 期 12, 页码 -

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AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.89.125126

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  1. Core Research Evolutional and Science and Technology program of the JST
  2. KAKENHI program of MEXT
  3. Tohoku University Evolution program

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We study transient dynamics of hole carriers injected into a Mott insulator with antiferromagnetic long-range order. This dynamical hole doping contrasts with chemical hole doping. The theoretical framework for the transient carrier dynamics is presented based on the two-dimensional t-J model. The time dependencies of the optical conductivity spectra, as well as the one-particle excitation spectra, are calculated based on the Keldysh Green's function formalism at zero temperature combined with the self-consistent Born approximation. In the early stage after dynamical hole doping, the Drude component appears, and then incoherent components originating from hole-magnon scattering start to grow. Fast oscillatory behavior owing to coherent magnon and slow relaxation dynamics are confirmed in the spectra. The time profiles are interpreted as doped bare holes being dressed by magnon clouds and relaxed into spin polaron quasiparticle states. The characteristic relaxation times for Drude and incoherent peaks strongly depend on the momentum of the dynamically doped hole and the exchange constant. Implications for recent pump-probe experiments are discussed.

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