期刊
PHYSICAL REVIEW B
卷 85, 期 22, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.85.224422
关键词
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资金
- LOEWE-Centre AdRIA
- DFG [SPP 1178]
- European Synchrotron Radiation Facility [HE-2379, HE-2848, HE-3567]
We have studied Ir spin and orbital magnetic moments in the double perovskites La2-xSrxCoIrO6 by x-ray magnetic circular dichroism. In La2CoIrO6, Ir4+ couples antiferromagnetically to the weak ferromagnetic moment of the canted Co2+ sublattice and shows an unusually large negative total magnetic moment (-0.38 mu(B)/f.u.) combined with strong spin-orbit interaction. In contrast, in Sr2CoIrO6, Ir5+ has a paramagnetic moment with almost no orbital contribution. A simple kinetic-energy-driven mechanism including spin-orbit coupling explains why Ir is susceptible to the induction of substantial magnetic moments in the double perovskite structure.
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