期刊
PHYSICAL REVIEW B
卷 86, 期 12, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.86.125102
关键词
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资金
- Air Force Office of Scientific Research (PECASE Award) [FA-9550-10-1-0026]
- National Science Foundation (CAREER Award) [EECS-0846466]
- Div Of Electrical, Commun & Cyber Sys
- Directorate For Engineering [0846466] Funding Source: National Science Foundation
Given growing interest in optical-frequency magnetic dipole transitions, we use intermediate coupling calculations to identify strong magnetic dipole emission lines that are well suited for experimental study. The energy levels for all trivalent lanthanide ions in the 4 f(n) configuration are calculated using a detailed free ion Hamiltonian, including electrostatic and spin-orbit terms as well as two-body, three-body, spin-spin, spin-other-orbit, and electrostatically correlated spin-orbit interactions. These free ion energy levels and eigenstates are then used to calculate the oscillator strengths for all ground-state magnetic dipole absorption lines and the spontaneous emission rates for all magnetic dipole emission lines including transitions between excited states. A large number of strong magnetic dipole transitions are predicted throughout the visible and near-infrared spectrum, including many at longer wavelengths that would be ideal for experimental investigation of magnetic light-matter interactions with optical metamaterials and plasmonic antennas.
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