期刊
PHYSICAL REVIEW B
卷 83, 期 18, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.83.184106
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资金
- UK Engineering and Physical Sciences Research Council
- EU [FP7, 228334]
- Ente Cassa di Risparmio di Firenze at LENS
- Spanish MALTA
- DOE/NNSA (CDAC), Army Research Office
- NSF [EAR-1015239]
- EPSRC [EP/J003999/1] Funding Source: UKRI
- Division Of Earth Sciences
- Directorate For Geosciences [1015239] Funding Source: National Science Foundation
- Engineering and Physical Sciences Research Council [EP/J003999/1] Funding Source: researchfish
High-resolution Raman spectroscopy of dense sodium reveals additonal low-energy lattice excitations in the three high-pressure phases cI 16, oP 8, and tI 19 from 108 to 178 GPa. The Raman-active lattice modes indicate profound changes of the chemical bonding in Na upon its transformation to an insulating state (hP 4 phase) at pressures above 178( 2) GPa. The calculated values of the valence electron localization maxima versus pressure provide insights into the experimentally observed solid-solid phase transitions and anomalous melting behavior of sodium.
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