期刊
PHYSICAL REVIEW B
卷 83, 期 24, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.83.245127
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资金
- Russian-Ukrainian [9-2010]
- FRSF of Ukraine [F29.1/014]
- German Science Foundation via DFG [LE 967/6-1, SPP 1458, TRR 80]
- grid cluster of Donetsk PhysTech NASU [N232]
- Swiss National Science Foundation [SNSF IZKOZ2_134161]
Polarized Raman-scattering spectra of nonsuperconducting, single-crystalline FeTe are investigated as a function of temperature. We have found a relation between the magnitude of ordered magnetic moments and the linewidth of A(1g) phonons at low temperatures. This relation is attributed to the intermediate spin state (S = 1) and the orbital degeneracy of Fe ions. Spin-phonon coupling constants have been estimated based on microscopic modeling using density functional theory and analysis of the local spin density. Our observations show the importance of orbital degrees of freedom for Fe-based superconductors with large ordered magnetic moments, while the small magnetic moment of Fe ions in some iron pnictides reflects the low spin state of Fe ions in those systems.
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