4.6 Article

Phonon-induced dephasing in single-wall carbon nanotubes

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PHYSICAL REVIEW B
卷 84, 期 11, 页码 -

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AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.84.115463

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  1. CNano IdF
  2. ANR agency

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We report on original nonlinear spectral hole-burning experiments in ensembles of single-wall carbon nanotubes. We have measured the temperature dependence of the excitonic homogeneous linewidth from 5 K up to room temperature. We show that the phonon-induced broadening in the weak coupling regime predominantly consists in pure dephasing. We present theoretical calculations of the exciton scattering rate due to phonon absorption within a one-dimensional framework for both excitons and phonons. We obtain a fair agreement with our experimental data and we discuss the specific properties of the exciton-phonon coupling in single-wall carbon nanotubes.

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