期刊
PHYSICAL REVIEW B
卷 84, 期 10, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.84.104202
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资金
- German BMBF [05KS4WWA/6, 05KS4VHA/4]
- Impuls- und Vernetzungsfonds of the Helmholtz Association [VH-NG-423]
- Department of Energy, Basic Energy Sciences [DE-AC02-05CH11231]
The electronic structure of aqueous NH3 and ND3 has been investigated using resonant inelastic soft x-ray scattering. Spectral features of different processes involving nuclear dynamics in the core-excited state can be identified. When exciting into the lowest core-excited state, we find a strong isotope effect and clear evidence for ultrafast proton dynamics. Furthermore, a strong vibronic coupling is observed and, in the case of aqueous NH3, a vibrational fine structure can be resolved.
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