期刊
PHYSICAL REVIEW B
卷 84, 期 18, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.84.184306
关键词
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资金
- Helmholtz University Young Investigator Group Lattices Dynamics in Emerging Functional Materials.
- NSF [DMR-0804719]
- 'Materials Sciences and Engineering Division', Office of Science, US Department of Energy
- Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy
The lattice dynamics of the filled skutterudite YbFe4Sb12 was studied by resonant ultrasound spectroscopy and an anomalous softening in the temperature dependence of the elastic constants at similar to 50 K was observed. This anomaly can not be explained by the dynamics of the filler, in contrast to other filled skutterudites. We have further investigated the origin of this anomaly using macroscopic and microscopic measurements. A rearrangement of the spectral weight of the Yb phonon states was observed in the temperature dependence of the density of phonon states, obtained by inelastic neutron scattering. We suggest that the anomaly is due to a change of the Yb valence state and that the anomaly and the phonon spectral weight rearrangement have the same origin.
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