期刊
PHYSICAL REVIEW B
卷 80, 期 3, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.80.033302
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资金
- Deutsche Forschungsgemeinschaft [SPP 1243]
Geometric symmetries cause orbital degeneracies in a molecule's spectrum. In a single-molecule junction, these degeneracies are lifted by various symmetry-breaking effects. We study quantum transport through such nanostructures with an almost degenerate spectrum. We show that the master equation for the reduced density matrix must be derived within the singular-coupling limit as opposed to the conventional weak-coupling limit. This results in strong signatures of the density matrix's off-diagonal elements in the transport characteristics.
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