期刊
PHYSICAL REVIEW B
卷 80, 期 15, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.80.155128
关键词
-
资金
- NSF [CHE-0650756]
We demonstrate the contribution of coherent excitation pathways in three-photon photoemission from Cu(001). We identify separate peaks in the photoelectron spectra as originating from two specific Cu d bands that are excited at different k points via the same unoccupied image-potential state. By model calculations we show that our experimental observations impose lower limits on the relevant Cu d-hole dephasing time on the order of 10-20 fs. Our findings suggest extensions to future studies in electronic structure mapping with tunable laboratory and free-electron laser sources, exploiting possible multiphoton resonances between occupied bulk and unoccupied surface states.
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