期刊
PHYSICAL REVIEW B
卷 80, 期 10, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.80.100407
关键词
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资金
- EPSRC-GB
- EC
- MAGMANet
- Department of Energy, Basic Energy Sciences [DE-AC02-07CH11358]
- Leverhulme Trust
- Royal Society
- FMU Professional Development Committee
- Alfred P. Sloan Foundation
We present tunnel diode oscillator (TDO) measurements of dynamic magnetic susceptibility, inelastic neutron-scattering (INS) measurements, and theoretical predictions based on quantum Monte Carlo (QMC) calculations for a magnetic molecule system, Cr12Cu2. The TDO measurements show not only ground-state level crossings (as can also be observed in low-temperature dc magnetization measurements) but also clear evidence of crossings between certain excited energy levels. These TDO results are in excellent agreement with our theoretical predictions for a Heisenberg Hamiltonian and are further confirmed by our INS measurements. Our present findings demonstrate that the TDO technique is a valuable magnetic spectroscopic tool for studying magnetic molecules, and that the QMC method is a valuable tool for predicting properties of computationally demanding systems such as Cr12Cu2.
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