4.6 Article

Effect of pressure on the quantum spin ladder material IPA-CuCl3

期刊

PHYSICAL REVIEW B
卷 78, 期 22, 页码 -

出版社

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.78.224409

关键词

high-pressure solid-state phase transformations; magnetic fluids; magnetic susceptibility; magnetic transitions; neutron diffraction

资金

  1. Division of Scientific User Facilities
  2. Office of Basic Energy Sciences
  3. U. S. Department of Energy [DE-AC05-00OR22725]
  4. National Science Foundation [DMR-9986442, DMR-0086210, DMR-0454672]

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Inelastic-neutron-scattering and bulk magnetic-susceptibility studies of the quantum S=1/2 spin ladder system (CH3)(2)CHNH3CuCl3 are performed under hydrostatic pressure. The pressure dependence of the spin gap Delta is determined. At P=1500 MPa it is reduced to Delta=0.79 meV from Delta=1.17 meV at ambient pressure. The results allow us to predict a soft-mode quantum phase transition in this system at P-c similar to 4 GPa. The measurements are complicated by the proximity of a structural phase transition that leads to a deterioration of the sample.

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