期刊
PHYSICAL REVIEW A
卷 89, 期 2, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevA.89.023420
关键词
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资金
- European Commission program ATTOFEL
- European Commission program CRISP
- European Commission program Laserlab Europe
- European COST Action [MPI1203-SKO, CM1204 XLIC]
- Greek funding program NSRF
- Advanced Grant of the European Research Council XCHEM [290853]
- European grant MC-RG ATTOTREND
- MICINN Project [FIS2010-15127]
- ERA-Chemistry Project [PIM2010EEC-00751]
Through frequency up-conversion of polarization-shaped, femtosecond laser pulses nonlinearly interacting with xenon atoms, energetic, broadband, coherent, XUV continuum radiation is generated. By exploiting the thus-formed short-duration XUV pulses, all the optically allowed excited states of H-2 are coherently populated. Nuclear and electronic 1-fs-scale dynamics are subsequently investigated by means of XUV-pump-XUV-probe measurements, which are compared to the results of ab initio calculations. The revealed dynamics reflects the intrinsic molecular behavior, as the XUV probe pulse hardly distorts the molecular potential.
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