4.6 Article

Subcycle laser control and quantum interferences in attosecond photoabsorption of neon

期刊

PHYSICAL REVIEW A
卷 87, 期 6, 页码 -

出版社

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevA.87.063413

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资金

  1. US Army Research Office
  2. National Science Foundation [1068604]
  3. Japan Society for the Promotion of Science [C24540421]
  4. HA-PACS Project for advanced interdisciplinary computational sciences by exa-scale computing technology
  5. Grants-in-Aid for Scientific Research [24540421] Funding Source: KAKEN
  6. Division Of Physics
  7. Direct For Mathematical & Physical Scien [1068604] Funding Source: National Science Foundation

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The dynamics of an atom in a strong infrared laser field (10(13) W/cm(2)) result in substantial changes to the field-free electronic energy levels, which can be probed on time scales shorter than the laser cycle using isolated attosecond pulses. Here, we measure the transient absorption of an isolated attosecond pulse by laser-dressed bound states of neon near the first ionization threshold. The observed subcycle changes in the absorption spectrum result from both laser-induced ac Stark shifts and from quantum interferences between different multiphoton excitation pathways. We further demonstrate the ability to experimentally turn off the quantum interference mechanism by eliminating one of the interfering pathways.

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