期刊
PHYSICAL REVIEW A
卷 86, 期 3, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevA.86.033401
关键词
-
资金
- Chemical Sciences, Geosciences, and Biosciences Division and the Advanced Photon Source by the Office of Basic Energy Sciences, Office of Science, US Department of Energy [DE-AC02-06CH11357]
Charge production, charge redistribution, and ion fragmentation are explored in the decay of a Xe K-shell vacancy in XeF2. Coincidence measurements of all ionic fragments in XeF2 provide evidence that an interatomic-Coulombic-decay-like (ICD-like) process plays a role in the cascade decay. The signature of the ICD-like process is an enhancement of the total number of electrons ejected as compared to the case of atomic Xe. The results indicate that the F atoms participate in the decay cascade within the first few femtoseconds after core-hole formation and that fragmentation begins during the decay process.
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